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1 article(s) from Polik, William F

Experimental and computational electrochemistry of quinazolinespirohexadienone molecular switches – differential electrochromic vs photochromic behavior

Eric W. Webb,
Jonathan P. Moerdyk,
Kyndra B. Sluiter,
Benjamin J. Pollock,
Amy L. Speelman,
Eugene J. Lynch,
William F. Polik and
Jason G. Gillmore

Beilstein J. Org. Chem. 2019, 15, 2473–2485, doi:10.3762/bjoc.15.240

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Scheme 1: PSHD photochromism [10].

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Figure 1: Proposed gating of sensitivity to photoinduced charge transfer by a photochromic photooxidant in wh...

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Scheme 2: QSHD photochromism [21].

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Figure 2: Cyclic voltammograms of a) 1b before irradiation or electrolysis (solid blue), b) 1b/2b after 25 sc...

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Figure 3: Cyclic voltammograms of a) 3b (with trace 5b) before irradiation or electrolysis (solid blue), b) 3b...

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Figure 4: Cyclic voltammograms of a) 3a before irradiation or electrolysis (solid blue), b) 3a + 5a after 25 ...

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Figure 5: ¹H NMR distinction between SW 3a, thermal/eLW 5a, and pLW 4a, in acetone-d₆, as observed a) before ...

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Figure 6: HOMO (MO 105, red and blue) and LUMO (MO 106, green and yellow) computed for 3a in its ground (S₀) ...

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Scheme 3: Proposed mechanism for differential formation of pLW (4) and eLW (5) from SW (3).

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Figure 7: Frontier orbital occupancies of relevant electronic states of 3a. Note: the photochemical excited s...

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Published 18 Oct 2019

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